I was wondering what the business case was for the switch. I'm evaluating both for a project of mine right now. (I use GXT for another project, but that won't fly for this one.)
I think it's interesting to see the different approaches used by jQuery and YUI. Plus if you know jQuery, you can get a good sense of YUI's style just by going down the list and comparing syntax.
This also pointed out a few things that YUI can do out of the box that jQuery can't, such as cross-domain requests via a flash helper.
PS: Is YUI3 gaining traction? Has features missing in jQuery? ...