going down the ios route is safest option.Pretty much in same boat as you taught my dad on online bill payments and banking in iPad . Set up a password manager and store all their personal information in there , make it available via touch id.
Chromebook and linux are still tech stuff which can not be handled by elderly.
Ublock Origin by gorhill is better, although the trouble with any ad-blocking plugin being used by non-technical people is that they will occasionally break a site and have no clue how to turn it off.